论文标题

在氧化的Cu/W界面处的大型自旋电荷互连的出现

Emergence of large spin-charge interconversion at an oxidized Cu/W interface

论文作者

Groen, Inge, Pham, Van Tuong, Ilić, Stefan, Choi, Won Young, Chuvilin, Andrey, Sagasta, Edurne, Vaz, Diogo C., Arango, Isabel C., Ontoso, Nerea, Bergeret, F. Sebastian, Hueso, Luis E., Tokatly, Ilya V., Casanova, Fèlix

论文摘要

旋转轨道设备可以通过利用自旋式互转换(SCI)来整合内存和逻辑,该互换(SCI)是通过设计和材料选择来优化的。在这些设备中,例如磁电旋转轨道(MESO)逻辑,界面是关键元素,因为它们可以禁止或促进设备中的自旋流以及具有旋转轨道耦合,从而导致界面SCI。在这里,我们研究了py/cu/w外侧自旋阀中SCI的起源,并量化其效率。 Cu和W电极之间界面的详尽表征可发现氧化层的存在(wo $ _x $)。我们确定SCI发生在Cu/wo $ _x $接口上,与温度无关的界面自旋传导电导率为$ g_ {|||} \ $ 20 $ 20 $ \ times $ 10 $ 10 $^{13}ω^{ - 1} m^{ - 1} m^{ - 2} $ andfacial spin-Charge $ charge toceitive $ capar-Charge $ capentivitive $ caperitive $ c} $ω^{ - 1} cm^{ - 1} $在10 k($ - $ 830 $ω^{ - 1} cm^{ - 1} $ 300 k)。这对应于逆Edelstein长度$λ_{IEE} = - $ 0.76 nm时的效率,在10 K(300 K时$ - $ 0.4 nm),比金属/金属和金属/金属/氧化物界面和散装重金属大。这种氧化界面上的大SCI效率是MESO逻辑设备中磁性读数的有前途的候选者。

Spin-orbitronic devices can integrate memory and logic by exploiting spin-charge interconversion (SCI), which is optimized by design and materials selection. In these devices, such as the magnetoelectric spin-orbit (MESO) logic, interfaces are crucial elements as they can prohibit or promote spin flow in a device as well as possess spin-orbit coupling resulting in interfacial SCI. Here, we study the origin of SCI in a Py/Cu/W lateral spin valve and quantify its efficiency. An exhaustive characterization of the interface between Cu and W electrodes uncovers the presence of an oxidized layer (WO$_x$). We determine that the SCI occurs at the Cu/WO$_x$ interface with a temperature-independent interfacial spin-loss conductance of $G_{||} \approx$ 20 $\times$ 10$^{13} Ω^{-1}m^{-2}$ and an interfacial spin-charge conductivity $σ_{SC}=-$1610 $Ω^{-1}cm^{-1}$ at 10 K ($-$830 $Ω^{-1}cm^{-1}$ at 300 K). This corresponds to an efficiency given by the inverse Edelstein length $λ_{IEE}=-$0.76 nm at 10 K ($-$0.4 nm at 300 K), which is remarkably larger than in metal/metal and metal/oxide interfaces and bulk heavy metals. The large SCI efficiency at such an oxidized interface is a promising candidate for the magnetic readout in MESO logic devices.

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