论文标题

手性液体的玻璃动力学

Glassy Dynamics in Chiral Fluids

论文作者

Debets, Vincent E., Löwen, Hartmut, Janssen, Liesbeth M. C.

论文摘要

手性活跃物质正在迅速增加兴趣,这是由于可以在例如活性颗粒的形状或自我刺激机制。尽管这已经导致了所谓的手性晶体的观察,但活跃的手性玻璃仍然在很大程度上没有探索。造成这种情况的一个可能原因可能是,相互作用主导玻璃动力学和主动运动的细节变得越来越小的相关性可能是幼稚的期望。在这里,我们证明,通过研究相互作用的手性活性布朗颗粒(CABP)的玻璃状动力学相反。我们证明,当将手性液推到玻璃状条件下时,它表现出高度不平凡的动力学,尤其是与标准的线性活性流体(如普通ABP)相比。尽管增加了复杂性,但我们仍然能够为所有已确定的动态制度提供全面合理化。最值得注意的是,我们引入了一种新的“锤击”机制,该机制是在高密度条件下快速旋转颗粒所特有的,可以使手性活性固体流畅。

Chiral active matter is enjoying a rapid increase of interest, spurred by the rich variety of asymmetries that can be attained in e.g. the shape or self-propulsion mechanism of active particles. Though this has already led to the observance of so-called chiral crystals, active chiral glasses remain largely unexplored. A possible reason for this could be the naive expectation that interactions dominate the glassy dynamics and the details of the active motion become increasingly less relevant. Here we show that quite the opposite is true by studying the glassy dynamics of interacting chiral active Brownian particles (cABPs). We demonstrate that when our chiral fluid is pushed to glassy conditions, it exhibits highly nontrivial dynamics, especially compared to a standard linear active fluid such as common ABPs. Despite the added complexity, we are still able to present a full rationalization for all identified dynamical regimes. Most notably, we introduce a new 'hammering' mechanism, unique to rapidly spinning particles in high-density conditions, that can fluidize a chiral active solid.

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