论文标题

各向同性熔体中的铁电列液滴

Ferroelectric Nematic Droplets in their Isotropic Melt

论文作者

Perera, Kelum, Nepal, Rony Saha Pawan, Dharmarathna, Rohan, Hossain, Md Sakhawat, Mostafa, Md, Adaka, Alex, Waroquet, Ronan, Twieg, Robert J., Jakli, Antal

论文摘要

一百多年前,对各向同性至铁电列液体过渡已经进行了研究,但其实验研究很少见。在这里,我们提出了与各向同性熔体共存的铁电液晶液滴的偏振光学显微镜研究和理论考虑。我们发现,只要有一个增加侧面液滴尺寸的空间,液滴的薄煎饼状形状比样品厚度薄。在液滴的中心,存在一个翼形的缺陷,其双折射为低,该缺陷垂直于弱平面电场,然后在较高场的两个处延伸并分裂。与缺陷运动和伸展平行,整个液滴以独立于液滴尺寸的速度沿电场漂移,并且与电场的振幅成正比。在场上增加到1V/mm之后,整个液滴会变形并随场振荡。这些观察结果使我们确定了极化场,并揭示了由于缺陷量周围极化而导致的一对正和负电荷。

The isotropic to ferroelectric nematic liquid transition had been theoretically studied over one hundred years ago, but its experimental studies are rare. Here we present polarizing optical microscopy studies and theoretical considerations of ferroelectric nematic liquid crystal droplets coexisting with the isotropic melt. We find that the droplets have flat pancake-like shapes that are thinner than the sample thickness as long as there is a room to increase the lateral droplet size. In the center of the droplets a wing shaped defect with low birefringence is present that moves perpendicular to a weak in-plane electric field, and then extends and splits in two at higher fields. Parallel to the defect motion and extension, the entire droplet drifts along the electric field with speed that is independent of the size of the droplet and is proportional to the amplitude of the electric field. After the field is increased above 1V/mm the entire droplet gets deformed and oscillates with the field. These observations led us to determine the polarization field and revealed the presence of a pair of positive and negative bound electric charge due to divergences of polarization around the defect volume.

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