论文标题

金属卤化物钙钛矿元素的电驱动激子 - 摩尔酮

Electrically driven exciton-polaritons in metal halide perovskite metatransistors

论文作者

Wang, Yutao, Tian, Jingyi, Klein, Maciej, Adamo, Giorgio, Ha, Son Tung, Soci, Cesare

论文摘要

通过光子和激子共振之间的强耦合产生的激子 - 摩尔体孔的电气注射是一个至关重要的里程碑,是扩大偏振器设备的重要里程碑,例如光学计算机,量子模拟器和无动力激光器。在这里,我们提出了一种新的方法,可以在电介质跨表面的连续体中单一构图在光发射晶体管的通道中单体图案的连续体中实现强耦合。激子 - 摩尔体是通过将元脉冲模式的栅极传输通道中的电注射的激子耦合来产生的,并衰减从晶体管顶部发出的光子中。多亏了元表面腔的高度,我们在钙钛矿膜的固有激素发射中获得了〜200 meV的大型狂犬分裂,并增强了极化的偏发射。此外,我们表明,可以通过改变控制激子的辐射重组区的源含量偏置来动态调节极性电致发光的方向性。我们认为,这种方法提供了一个新的平台,可以在电气注射下在分散工程的光子腔中研究较强的光 - 物质相互作用,并为解决溶液处理的电泵送偏光量激光器铺平了道路。

Achieving electrical injection of exciton-polaritons, half-light, half-matter quasiparticles arising from the strong coupling between photonic and excitonic resonances, is a crucial milestone to scale up polaritonic devices such as optical computers, quantum simulators and inversionless lasers. Here we present a new approach to achieve strong coupling between electrically injected excitons and photonic bound states in the continuum of a dielectric metasurface monolithically patterned in the channel of a light-emitting transistor. Exciton-polaritons are generated by coupling electrically injected excitons in the gate-induced transport channel with a Bloch mode of the metasurface, and decay into photons emitted from the top surface of the transistor. Thanks to the high-finesse of the metasurface cavity, we achieve a large Rabi splitting of ~200 meV and more than 50-fold enhancement of the polaritonic emission over the intrinsic excitonic emission of the perovskite film. Moreover, we show that the directionality of polaritonic electroluminescence can be dynamically tuned by varying the source-drain bias which controls the radiative recombination zone of the excitons. We argue that this approach provides a new platform to study strong light-matter interaction in dispersion engineered photonic cavities under electrical injection, and paves the way to solution-processed electrically pumped polariton lasers.

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