论文标题

$ω-2Ω$ thres-threshold电离的半经典强场延迟

Semiclassical strong-field theory of phase delays in $ω-2ω$ above-threshold ionization

论文作者

Arbó, Diego G., López, Sebastián D., Burgdörfer, Joachim

论文摘要

最近在$ω-2Ω$设置中探索了原子高于阈值电离的相位和时间延迟[Zipp等,Optica 1,361(2014)]。从Argon弹出的波袋的阶段是强$2Ω$脉冲的探测,这是较弱的$ω$探针脉冲的相对相的函数。求解时间依赖性Schrödinger方程(TDSE)的数值模拟显示出对$ω$和$2Ω$字段之间相对相位的双重差分动量分布的敏感依赖性。此外,发现了提取相延迟在探针脉冲强度上的出人意料的强烈变化。我们提出了在$ω-2Ω$设置中电子发射中相位延迟的半经典强场描述,并将其应用于原子氢。包括$2Ω$泵和$ω$探针字段的非扰动效果。半古典描述允许追踪阶段延迟到两种彩色激光场的颞单元单元内发射时间内发射时发射之间的路径干扰。我们发现半经典鞍点近似,完整的强场近似(SFA)和先前适用于探针场扰动限制的结果之间的良好一致性。我们表明,类似兔子的相位延迟的扰动描述会破坏更强的场和更高的电子发射。在此制度中,电离信号的表征需要相位延迟的整个集合{$Δ_i(e)$},$ i = 1,2,\ ldots $涉及干扰路径中强$2Ω$场的光子数量的差异。 SFA和TDSE计算之间的比较也揭示了库仑场的影响,即使在这种强场景中。

Phase and time delays of atomic above-threshold ionization were recently experimentally explored in an $ω-2ω$ setting [Zipp et al, Optica 1, 361 (2014)]. The phases of wavepackets ejected from argon by a strong $2ω$ pulse were probed as a function of the relative phase of a weaker $ω$ probe pulse. Numerical simulations solving the time-dependent Schrödinger equation (TDSE) displayed a sensitive dependence of the doubly differential momentum distribution on the relative phase between the $ω$ and $2ω$ fields. Moreover, a surprisingly strong variation of the extracted phase delays on the intensity of the probe pulse was found. We present a semiclassical strong-field description of the phase delays in the emission of electrons in an $ω-2ω$ setting and apply it to atomic hydrogen. Non-perturbative effects in both the $2ω$ pump and the $ω$ probe field are included. The semiclassical description allows tracing phase delays to path interferences between emission during different points in time of emission within the temporal unit cell of the two-color laser field. We find good agreement between the semiclassical saddle-point approximation, the full strong field approximation (SFA), and previous results applicable in the perturbative limit of probe fields. We show that the RABBIT-like perturbative description of phase delays breaks down for stronger fields and higher-energy electron emission. In this regime, characterization of the ionization signal requires an entire ensemble of phase delays {$δ_i(E)$} with $i=1,2,\ldots$ the difference in photon numbers of the strong $2ω$ field involved in the interfering paths. Comparison between SFA and TDSE calculations reveals the influence of the Coulomb field even in this strong-field scenario.

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