论文标题
石墨上的物理学金簇的结构润滑及其分解:边界条件和接触线的作用
Structural lubricity of physisorbed gold clusters on graphite and its breakdown: Role of boundary conditions and contact lines
论文作者
论文摘要
使用分子动力学模拟了吸附在石墨底物上的金色平板的滑动运动。兴趣的中心量是平均横向力,即动力学摩擦而不是最大侧向力,与静态摩擦相关。对于大多数设置,我们发现Stokesian阻尼可抵抗滑动。但是,如果将三个石墨层的底层层保持在零应力而不是零位移时,则观察到有限宽度平板平行于扶手椅方向平行于扶手椅方向平行于扶手椅方向的有限宽度平板的摩擦(库仑)摩擦。尽管由此产生的动力摩擦仍然低于结构润滑接触的典型(保守)力的不稳定的波动所产生的噪声,但导致库仑摩擦的不稳定性的性质可以表征为莫伊尔(quasi-Dosifiction)的摩rus摩尔模式的莫伊尔(Moiré)模式,该模式是由正常位移所形成的莫伊尔(Moiré)模式。看来,当接触线平行于扶手椅而不是锯齿形方向时,石墨与第二金层的相互作用是导致界面中发生的对称破裂的原因。
The sliding motion of gold slabs adsorbed on a graphite substrate is simulated using molecular-dynamics. The central quantity of interest is the mean lateral force, i.e., the kinetic friction rather than the maximum lateral forces, which correlate with the static friction. For most set-ups, we find Stokesian damping to resist sliding. However, velocity-insensitive (Coulomb) friction is observed for finite-width slabs sliding parallel to the armchair direction if the bottommost layer of the three graphite layers is kept at zero stress rather than at zero displacement. Although the resulting kinetic friction remain much below the noise produced by the erratic fluctuations of (conservative) forces typical for structurally lubric contacts, the nature of the instabilities leading to Coulomb friction could be characterized as quasi-discontinuous dynamics of the Moiré patterns formed by the normal displacements near a propagating contact line. It appears that the interaction of the graphite with the second gold layer is responsible for the symmetry breaking occurring in the interface when a contact line moves parallel to the armchair rather than to the zigzag direction.