论文标题

新的人造光合系统耦合光伏电催化与光热催化

A new artificial photosynthetic system coupling photovoltaic electrocatalysis with photothermal catalysis

论文作者

Li, Yaguang, Meng, Fanqi, Bai, Xianhua, Yuan, Dachao, San, Xingyuan, Liang, Baolai, Fu, Guangsheng, Wang, Shufang, Gu, Lin, Meng, Qingbo

论文摘要

在这项工作中,我们提出了一种新型的人造光合作用范式,通过整合光伏电解水拆分设备和太阳能加热CO2氢化设备,成功实现了1 Sun驱动的19.4%Solar到CO的生产(2.2.7乘以CO的较高的艺术)的ARTTHY ARTTHS SYSERNE,可通过平方米(M2)水平可扩展的生产产生可伸缩的生产(2.4%驱动的19.4%驱动的Artthy Artshized Artshize Artinth Artsive of Artsive Artssive of Artsive Artshized Artshige of Artsive Artsive Artshized Artshige(2.2.7) (相当于报告的人工光合系统的1/7)。此外,以1.268 m2的规模为户外人造光合示范表现出每天258.4升的CO生成量,冬季的CO生产的STC约为15.5%,可以通过销售Co在833 Suuny日内收回成本。

In this work, we present a novel artificial photosynthetic paradigm with square meter (m2) level scalable production by integrating photovoltaic electrolytic water splitting device and solar heating CO2 hydrogenation device, successfully achieving the synergy of 1 sun driven 19.4% solar to chemical energy efficiency (STC) for CO production (2.7 times higher than state of the art of large-sized artificial photosynthetic systems) with a low cost (equivalent to 1/7 of reported artificial photosynthetic systems). Furthermore, the outdoor artificial photosynthetic demonstration with 1.268 m2 of scale exhibits the CO generation amount of 258.4 L per day, the STC of ~15.5% for CO production in winter, which could recover the cost within 833 suuny days of operation by selling CO.

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