论文标题

理论指导的MNPT磁性演化调查

Theory-guided investigation on magnetic evolution of MnPt$_{5-x}$Pd$_x$P and discovery of anti-CeCoIn$_5$-type ferromagnetic MnPd$_5$P

论文作者

Mudiyanselage, Ranuri S. Dissanayaka, Kang, Chang-Jong, Wei, Kaya, Shu, Zhixue, Kong, Tai, Baumbach, Ryan, Kotliar, Gabriel, Xie, Weiwei

论文摘要

我们报告了抗抗铁磁剂到反115型MNPT $ _ {5-x} $ pd $ _x $ p($ x $ = 1,2,2.5,3,4和5)的磁变化,并发现了一个新的稀有稀有的Ferromagnet $ _-5 $。使用高温固态方法合成家族化合物,并表征在抗蛋白质$ _5 $中结晶,其空间组P4/mmm具有二维分层结构特征。磁性测量值表明,从MNPT的倾斜A型抗铁磁铁中排序的化合物$ _5 $ P $ _5 $ P以高于室温的超过室温,并在MNPD $ _5 $ p的不同程度上以不同程度的胁迫和磁性矩来减少旋转孔孔偶联。与151个MN家族(PT/PD)$ _ 5 $(P/AS)相比,已经分析了MNPT $ _ {5-X} $ PD $ _X $ P的结果,以了解复杂的结构 - 磁性关系。

We report the magnetic changes from canted antiferromagnetic to ferromagnetic orderings in anti-115-type MnPt$_{5-x}$Pd$_x$P ($x$ = 1, 2, 2.5, 3, 4, and 5) and the discovery of a new rare-earth-free ferromagnet, MnPd$_5$P by both theoretical prediction and experimental investigation. The family compounds were synthesized using high temperature solid state method and characterized to crystalize in the anti-CeCoIn$_5$ type with the space group P4/mmm exhibiting a two-dimensional layered structural feature. The magnetic property measurements indicate that the compounds ordered from canted A-type antiferromagnet in MnPt$_5$P to ferromagnet above the room temperature with varying degrees of coercivity and magnetic moments in MnPd$_5$P by reducing the spin orbital coupling. The results of the MnPt$_{5-x}$Pd$_x$P have been analyzed in comparison to the other candidates of the 151 family of Mn(Pt/Pd)$_5$(P/As) to understand the complex structure-magnetism relationships.

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