论文标题

由粘弹性培养基引起的活性布朗运动与记忆延迟

Active Brownian motion with memory delay induced by a viscoelastic medium

论文作者

Sprenger, Alexander R., Bair, Christian, Löwen, Hartmut

论文摘要

到目前为止,主动布朗运动是一个良好的模型,用于描述牛顿液中介镜自行颗粒的运动。在广义的langevin方程的基础上,我们提出了一个分析框架,用于主动布朗运动的分析框架,并假设具有时间依赖性的摩擦核,用于转化和定向的自由度,以说明粘弹性介质的时间延迟响应。获得方向相关函数,平均位移和均方位移的分析结果,我们特别评估了麦克斯韦流体,其特征在于核的特征,该核会及时呈指数衰减。此外,我们确定了记忆引起的延迟在有效的自我螺旋力和粒子方向之间,我们根据特殊的动态相关函数进行了量化。原则上,我们可以在各种粘弹性环境(例如聚合物溶液)中为活性胶体粒子验证我们的预测。

By now active Brownian motion is a well-established model to describe the motion of mesoscopic self-propelled particles in a Newtonian fluid. On the basis of the generalized Langevin equation, we present an analytic framework for active Brownian motion with memory delay assuming time-dependent friction kernels for both translational and orientational degrees of freedom to account for the time-delayed response of a viscoelastic medium. Analytical results are obtained for the orientational correlation function, mean displacement and mean-square displacement which we evaluate in particular for a Maxwell fluid characterized by a kernel which decays exponentially in time. Further, we identify a memory induced delay between the effective self-propulsion force and the particle orientation which we quantify in terms of a special dynamical correlation function. In principle our predictions can be verified for an active colloidal particle in various viscoelastic environments such as a polymer solution.

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