论文标题
Srruo $ _3 $,caruo $ _3 $和sr $ _2 $ ruo $ _4 $ thin Fimss中的分离运输放松量表和频带散射
Separated transport relaxation scales and interband scattering in SrRuO$_3$, CaRuO$_3$, and Sr$_2$RuO$_4$ thin films
论文作者
论文摘要
在某些密切相关的金属中观察到的异常电荷转运提出了有关Landau Fermi液体理论的普遍适用性的问题。对于普通金属的相干温度$ t_ {fl} $通常是在电阻率中观察到$ t^2 $的温度。在此温度以下,预计具有定义明确的准粒子的费米液体。然而,尽管经常观察到$ t^2 $ dc的电阻率,但在鲁德斯顿 - 帕普尔家族中的金属鲜明是在Ruddlesden-Popper家族中经常显示出非干燥的低能量光学电导率和不寻常的$ω/T $缩放。本文中,我们报告了几种不同高质量金属鲜花纯酸酯薄膜的时间域THZ光谱测量值,并表明可以用更传统的术语来解释光学电导率。在所有材料中,电导率在低温下具有两阵峰线形状,在较高温度下的分频器均具有分频器到单干峰线。两个组分的低温电导率表示不同传导通道的两个良好分离的当前弛豫率。我们讨论了分离速率的三种特殊可能性:(a)强烈依赖能量的非弹性散射; (b)一个几乎保存的伪符号操作员,与电流重叠,从而导致较窄的drude峰; (c)存在多个传导通道,这些通道在较高温度下经历了跨界的跨界散射。这些情况都不需要异国情调的准颗粒。结果可能会深入了解Hund耦合在确定这些材料中带偶联的可能意义。我们的结果还显示了了解这类材料中对Matthiessen统治的违规途径,并与费米液体中的“ Gurzhi”扩展关系的偏差。
The anomalous charge transport observed in some strongly correlated metals raises questions as to the universal applicability of Landau Fermi liquid theory. The coherence temperature $T_{FL}$ for normal metals is usually taken to be the temperature below which $T^2$ is observed in the resistivity. Below this temperature, a Fermi liquid with well-defined quasiparticles is expected. However, metallic ruthenates in the Ruddlesden-Popper family, frequently show non-Drude low-energy optical conductivity and unusual $ω/T$ scaling, despite the frequent observation of $T^2$ dc resistivity. Herein we report time-domain THz spectroscopy measurements of several different high-quality metallic ruthenate thin films and show that the optical conductivity can be interpreted in more conventional terms. In all materials, the conductivity has a two-Drude peak lineshape at low temperature and a crossover to a one-Drude peak lineshape at higher temperatures. The two-component low-temperature conductivity is indicative of two well-separated current relaxation rates for different conduction channels. We discuss three particular possibilities for the separation of rates: (a) Strongly energy-dependent inelastic scattering; (b) an almost-conserved pseudomomentum operator that overlaps with the current, giving rise to the narrower Drude peak; (c) the presence of multiple conduction channels that undergoes a crossover to stronger interband scattering at higher temperatures. None of these scenarios require the existence of exotic quasiparticles. The results may give insight into the possible significance of Hund's coupling in determining interband coupling in these materials. Our results also show a route towards understanding the violation of Matthiessen's rule in this class of materials and deviations from the "Gurzhi" scaling relations in Fermi liquids.