论文标题

近距Kitaev量子旋转液体$α$ -rucl $ _3 $中的巨型声子异常

Giant Phonon Anomalies in the Proximate Kitaev Quantum Spin Liquid $α$-RuCl$_3$

论文作者

Li, H., Zhang, T. T., Said, A., Fabbris, G., Mazzone, D. G., Yan, J. Q., Mandrus, D., Halasz, G. B., Okamoto, S., Murakami, S., Dean, M. P. M., Lee, H. N., Miao, H.

论文摘要

Kitaev量子自旋液体体现了纠缠的拓扑状态,为此,预测了两种分数低能激发的口味:流动的Majorana fermion和Z2量规通量。由于它们的分数量子数和非本地性,对这些激发的检测仍然具有挑战性。最近有人提出,通过新型的分数激发 - 偶联耦合,将分数激发的指纹编码在Kitaev量子旋转液体的声子光谱中。在这里,我们使用MEV分辨率的非弹性X射线散射在$α$ -RUCL3中发现了这种效果。在高温下,我们发现了隔开的光学声子拦截3至7 MeV之间的横向声音子。温度降低后,光子声子在Kitaev Energy(JK〜8 MEV)附近显示出较大的强度增强,与Z2量规通量量表附近的巨大声音声子软化相吻合。这种分数激发引起的声子异常发现了$α$ -RUCL3中量子热厅效应的关键成分,并展示了一种原理证明方法,可检测拓扑量子材料中的分数激发。

The Kitaev quantum spin liquid epitomizes an entangled topological state, for which two flavors of fractionalized low-energy excitations are predicted: the itinerant Majorana fermion and the Z2 gauge flux. Detection of these excitations remains challenging, because of their fractional quantum numbers and non-locality. It was proposed recently that fingerprints of fractional excitations are encoded in the phonon spectra of Kitaev quantum spin liquids through a novel fractional-excitation-phonon coupling. Here, we uncover this effect in $α$-RuCl3 using inelastic X-ray scattering with meV resolution. At high temperature, we discover interlaced optical phonons intercepting a transverse acoustic phonon between 3 and 7 meV. Upon decreasing temperature, the optical phonons display a large intensity enhancement near the Kitaev energy, JK~8 meV, that coincides with a giant acoustic phonon softening near the Z2 gauge flux energy scale. This fractional excitation induced phonon anomalies uncover the key ingredient of the quantum thermal Hall effect in $α$-RuCl3 and demonstrates a proof-of-principle method to detect fractional excitations in topological quantum materials.

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