论文标题

无序超导体中的集体模式的第三次谐波生成

Third harmonic generation from collective modes in disordered superconductors

论文作者

Seibold, G., Udina, M., Castellani, C., Benfatto, L.

论文摘要

在常规和非常规超导体中具有强大THZ领域的最新实验清楚地证明了低于超导温度$ T_C $的第三次谐波一代。它的解释挑战了实质性的理论工作,旨在建立准粒子激发和集体模式在触发这种共振反应方面的相对效率。在这里,我们通过实施时间依赖的Bogoljubov De-gennes方法来计算非线性电流,双重旨在非扰动局部疾病的效果,并包括所有集体模式的贡献,即超导幅度振幅(HIGGS)和相位波动和充电波动。我们表明,与以前的工作一致,已经处于小疾病中,准粒子反应主要由顺磁效应主导。我们进一步证明,顺磁过程还介导了所有集体模式的响应,并具有大量电荷/相波动的贡献。到目前为止,这些过程已被忽略了,结果占据了强障碍的三阶电流。此外,我们表明,混乱会强烈影响非线性响应的极化依赖性,而清洁和无序情况之间的差异很大。我们的结果尤其与丘比特的最新实验相关,丘比特的最新实验是由我们的晶格模型重现的第一个近似值。

Recent experiments with strong THz fields in both conventional and unconventional superconductors have clearly evidenced a marked third-harmonic generation below the superconducting temperature $T_c$. Its interpretation challenged substantial theoretical work aimed at establishing the relative efficiency of quasiparticle excitations and collective modes in triggering such a resonant response. Here we compute the non-linear current by implementing a time-dependent Bogoljubov de-Gennes approach, with the twofold aim to account non-perturbatively for the effect of local disorder, and to include the contribution of all collective modes, i.e. superconducting amplitude (Higgs) and phase fluctuations, and charge fluctuations. We show that, in agreement with previous work, already at small disorder the quasiparticle response is dominated by paramagnetic effects. We further demonstrate that paramagnetic processes mediate also the response of all collective modes, with a substantial contribution of charge/phase fluctuations. These processes, which have been overlooked so far, turn out to dominate the third-order current at strong disorder. In addition, we show that disorder strongly influences the polarization dependence of the non-linear response, with a marked difference between the clean and the disordered case. Our results are particularly relevant for recent experiments in cuprates, whose band structure is in a first approximation reproduced by our lattice model.

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