论文标题

外在卤化物钙钛矿的特殊相相一致性长度

Extraordinary Phase Coherence Length in Epitaxial Halide Perovskites

论文作者

Nasyedkin, K., King, I., Zhang, L., Chen, P., Wang, L., Staples, R. J., Lunt, R. R., Pollanen, J.

论文摘要

在从太阳能收集到计算和光发射的广泛应用中,无机卤化物钙钛矿已成为有前途的平台。卤化物钙钛矿的外在薄膜生长的最近出现使得基于此类材料研究了低维量子电子设备成为可能。这项研究利用了卤化物钙钛矿的蒸气相外延的进步,以对单域剖腹碘化物(CSSSNI $ _3 $)的外延薄膜进行低温磁转运测量。低场磁场具有相干量子干扰效应和自旋轨道耦合的特征。这些弱的抗本地化测量结果揭示了该系统中电荷载体的微米尺度低温相一致性长度。结果表明,外延卤化物钙钛矿异质结构是研究长相干量子电子效应以及旋转三位型和自旋轨道货币学中的潜在应用的有前途的平台。

Inorganic halide perovskites have emerged as a promising platform in a wide range of applications from solar energy harvesting to computing, and light emission. The recent advent of epitaxial thin film growth of halide perovskites has made it possible to investigate low-dimensional quantum electronic devices based on this class of materials. This study leverages advances in vapor-phase epitaxy of halide perovskites to perform low-temperature magnetotransport measurements on single-domain cesium tin iodide (CsSnI$_3$) epitaxial thin films. The low-field magnetoresistance carries signatures of coherent quantum interference effects and spin-orbit coupling. These weak anti-localization measurements reveal a micron-scale low-temperature phase coherence length for charge carriers in this system. The results indicate that epitaxial halide perovskite heterostructures are a promising platform for investigating long coherent quantum electronic effects and potential applications in spintronics and spin-orbitronics.

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