论文标题
通过破坏旋转对称性的洪德金属中电荷不稳定性的增强
Enhancement of charge instabilities in Hund's metals by the breaking of rotational symmetry
论文作者
论文摘要
我们分析了描述Hund金属的多轨哈驼峰模型,重点是无处不在的电荷不稳定性发生,这是由发散/负电子压缩性信号,这是从半填充的Mott绝缘子的一系列掺杂,与Hund Metals和正常金属之间的前沿相对应。我们表明,旋转不变性的破裂有利于这种不稳定性:相互作用中的自旋 - 扭转型和轨道之间的晶体场分裂使不稳定性区域扩展到较大的兴奋剂,从而使其与基于铁的超导体等真实材料相关。这些观察结果帮助我们建立了这种不稳定的发生和程度的连贯图片。我们将其追溯到Hund金属中当地自由度的部分冻结,从而降低了允许的局部配置,从而减少了准粒子巡回术。在洪德金属边界上发生的未重新释放的突然性可以直接连接到电子动能的快速变化,从而与可压缩性的增强和差异有关。
We analyze multi-orbital Hubbard models describing Hund's metals, focusing on the ubiquitous occurrence of a charge instability, signalled by a divergent/negative electronic compressibility, in a range of doping from the half-filled Mott insulator corresponding to the frontier between Hund's and normal metals. We show that the breaking of rotational invariance favors this instability: both spin-anisotropy in the interaction and crystal-field splitting among the orbitals make the instability zone extend to larger dopings, making it relevant for real materials like iron-based superconductors. These observations help us build a coherent picture of the occurrence and extent of this instability. We trace it back to the partial freezing of the local degrees of freedom in the Hund's metal, which reduces the allowed local configurations and thus the quasiparticle itinerancy. The abruptness of the unfreezing happening at the Hund's metal frontier can be directly connected to a rapid change in the electronic kinetic energy and thus to the enhancement and divergence of the compressibility.