论文标题

魔术角石墨烯中Pomeranchuk效应的熵证据

Entropic evidence for a Pomeranchuk effect in magic angle graphene

论文作者

Rozen, Asaf, Park, Jeong Min, Zondiner, Uri, Cao, Yuan, Rodan-Legrain, Daniel, Taniguchi, Takashi, Watanabe, Kenji, Oreg, Yuval, Stern, Ady, Berg, Erez, Jarillo-Herrero, Pablo, Ilani, Shahal

论文摘要

在1950年代,Pomeranchuk预测,违反直觉,由于固相中的高过量自旋熵,液体3HE可能在加热后固化。在这里,使用局部和全局电子熵和可压缩性测量值,我们表明在魔术角扭曲的双层石墨烯中发生了类似的效果。在每个moir'e单位电池的一个电子填充物附近,我们观察到电子熵的急剧增加到人均约1KB。这种大量的熵被平面磁场淬灭,指向其磁性。压缩性随着电子密度的函数而急剧下降,这与将费米水平重置回到狄拉克点附近相关,标志着两个阶段之间的清晰边界。我们将此跳跃映射为电子密度,温度和磁场的函数。这揭示了一个相图,该相图与pomeranchuk样温度和现场驱动的温度和野外驱动的过渡是一致的,从低进入电子液体到具有近乎无磁矩的高渗透相关状态。相关状态具有看似矛盾的特性的异常组合,有些与巡回电子相关,例如没有热力学间隙,金属性和类似狄拉克的可压缩性以及与局部矩相关的其他相关性,例如,诸如大熵及其与磁场的消失。此外,表征这两组属性的能量尺度截然不同:尽管可压缩性在t〜30k处的跳动量,但磁激发的带宽为〜3k或更小。新相关状态的杂种性质和能量尺度的较大分离对扭曲双层石墨烯中相关状态物理的关键意义。

In the 1950's, Pomeranchuk predicted that, counterintuitively, liquid 3He may solidify upon heating, due to a high excess spin entropy in the solid phase. Here, using both local and global electronic entropy and compressibility measurements, we show that an analogous effect occurs in magic angle twisted bilayer graphene. Near a filling of one electron per moir'e unit cell, we observe a dramatic increase in the electronic entropy to about 1kB per unit cell. This large excess entropy is quenched by an in-plane magnetic field, pointing to its magnetic origin. A sharp drop in the compressibility as a function of the electron density, associated with a reset of the Fermi level back to the vicinity of the Dirac point, marks a clear boundary between two phases. We map this jump as a function of electron density, temperature, and magnetic field. This reveals a phase diagram that is consistent with a Pomeranchuk-like temperature- and field-driven transition from a low-entropy electronic liquid to a high-entropy correlated state with nearly-free magnetic moments. The correlated state features an unusual combination of seemingly contradictory properties, some associated with itinerant electrons, such as the absence of a thermodynamic gap, metallicity, and a Dirac-like compressibility, and others associated with localized moments, such as a large entropy and its disappearance with magnetic field. Moreover, the energy scales characterizing these two sets of properties are very different: whereas the compressibility jump onsets at T~30K, the bandwidth of magnetic excitations is ~3K or smaller. The hybrid nature of the new correlated state and the large separation of energy scales have key implications for the physics of correlated states in twisted bilayer graphene.

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