论文标题

具有无限层结构的超导praseodymim镍

A superconducting praseodymium nickelate with infinite layer structure

论文作者

Osada, Motoki, Wang, Bai Yang, Goodge, Berit H., Lee, Kyuho, Yoon, Hyeok, Sakuma, Keita, Li, Danfeng, Miura, Masashi, Kourkoutis, Lena F., Hwang, Harold Y.

论文摘要

长期以来,已经研究了多种氧化氧化物化合物,以表现出各种相关电子现象。最近,在纳米级无限层镍薄膜中观察到了超导性,该薄膜的Nd $ _ {0.8} $ sr $ _ {0.2} $ nio $ _2 $,在perovskite tooptactic降低的Srtio $ _3 $ siderates上表现出稳定,从perovskite perovskite the perovskite copertor阶段稳定。在这里,我们介绍prnio $ _2 $薄膜的综合和属性在srtio $ _3 $上。掺杂pr $ _ {0.8} $ sr $ _ {0.2} $ nio $ _2 $,我们观察到超导性,过渡温度为7-12 k,在2 k的334 ka/cm $ $^2 $的2 k时,稳健的临界电流密度可强。这些发现表明,无限层镍的超导性对稀土4 $ f $配置的细节相对不敏感。此外,它们激发了基于二维Nio $ _2 $飞机对更广泛的化合物的探索,这将使对超导和正常状态特性及其潜在机制进行系统的研究。

A variety of nickel oxide compounds have long been studied for their manifestation of various correlated electron phenomena. Recently, superconductivity was observed in nanoscale infinite layer nickelate thin films of Nd$_{0.8}$Sr$_{0.2}$NiO$_2$, epitaxially stabilized on SrTiO$_3$ substrates via topotactic reduction from the perovskite precursor phase. Here we present the synthesis and properties of PrNiO$_2$ thin films on SrTiO$_3$. Upon doping in Pr$_{0.8}$Sr$_{0.2}$NiO$_2$, we observe superconductivity with a transition temperature of 7-12 K, and robust critical current density at 2 K of 334 kA/cm$^2$. These findings indicate that superconductivity in the infinite layer nickelates is relatively insensitive to the details of the rare earth 4$f$ configuration. Furthermore, they motivate the exploration of a broader family of compounds based on two-dimensional NiO$_2$ planes, which will enable systematic investigation of the superconducting and normal state properties and their underlying mechanisms.

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