论文标题

在环境条件下,使用扫描微波阻抗显微镜对Moiré晶格和上层建筑的超高分辨率成像

Ultra-high-resolution imaging of moiré lattices and superstructures using scanning microwave impedance microscopy under ambient conditions

论文作者

Lee, Kyunghoon, Utama, M. Iqbal Bakti, Kahn, Salman, Samudrala, Appalakondaiah, Leconte, Nicolas, Yang, Birui, Wang, Shuopei, Watanabe, Kenji, Taniguchi, Takashi, Zhang, Guangyu, Weber-Bargioni, Alexander, Crommie, Michael, Ashby, Paul D., Jung, Jeil, Wang, Feng, Zettl, Alex

论文摘要

具有略有不同晶格矢量层的二维异质结构显示出一种新的周期性结构,称为Moire Lattices。 Moire Grattice地层提供了一种强大的新方法,以设计二维材料的电子结构,以实现新颖的相关和拓扑现象。此外,Moire Lattices的上层建筑可以从多个未对准的晶格向量或不均匀应变分布中出现,该分布在电子带结构设计中提供了额外的自由度。 Moire晶格和上层建筑的高分辨率成像对于定量了解新兴Moire物理学至关重要。在这里,我们报告了在环境条件下,使用扫描微波阻抗显微镜的超高分辨率实现在环境条件下在各种基于石墨烯的样品中对Moire晶格和上层建筑的纳米级成像。我们表明,尽管扫描探针尖端的总半径约为100 nm,但可以实现局部电导率曲线的超高空间分辨率,但可以实现比5 nm更好的空间分辨率。这种分辨率的增强不仅使魔术角扭曲的双重双层石墨烯和复合超级摩尔晶格可以直接可视化Moire晶格,而且还允许设计道路,可以设计出人工合成新颖的Moire上层结构,例如来自Interplay的Kagome Moire等新型Moire上层结构,并在扭曲的地铁和Hexagonal boronnitriderilide中进行了超级重塑。

Two-dimensional heterostructures with layers of slightly different lattice vectors exhibit a new periodic structure known as moire lattices. Moire lattice formation provides a powerful new way to engineer the electronic structure of two-dimensional materials for realizing novel correlated and topological phenomena. In addition, superstructures of moire lattices can emerge from multiple misaligned lattice vectors or inhomogeneous strain distribution, which offers an extra degree of freedom in the electronic band structure design. High-resolution imaging of the moire lattices and superstructures is critical for quantitative understanding of emerging moire physics. Here we report the nanoscale imaging of moire lattices and superstructures in various graphene-based samples under ambient conditions using an ultra-high-resolution implementation of scanning microwave impedance microscopy. We show that, quite remarkably, although the scanning probe tip has a gross radius of ~100 nm, an ultra-high spatial resolution in local conductivity profiles better than 5 nm can be achieved. This resolution enhancement not only enables to directly visualize the moire lattices in magic-angle twisted double bilayer graphene and composite super-moire lattices, but also allows design path toward artificial synthesis of novel moire superstructures such as the Kagome moire from the interplay and the supermodulation between twisted graphene and hexagonal boron nitride layers.

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