论文标题

fe $ _ {1+y}的电子相图

Electronic phase diagram of Fe$_{1+y}$Te$_{1-x}$Se$_{x}$ revealed by magnetotransport measurements

论文作者

Watanabe, Takao, Otsuka, Takumi, Hagisawa, Shotaro, Koshika, Yuta, Adachi, Shintaro, Usui, Tomohiro, Sasaki, Nae, Sasaki, Seya, Yamaguchi, Shunpei, Uezono, Yu, Nakanishi, Yoshiki, Yoshizawa, Masahito, Kimura, Shojiro

论文摘要

在基于Fe的超导体中,Fe $ _ {1+y} $ te $ _ {1-x} $ se $ _ {x} $是独一无二的,因为它的晶体结构是最简单的,并且电子相关级别是最强的,因此对于调查掺杂($ x $) - 温度($ t $)的相位很重要。但是,目前不可避免地将多余的FE纳入了超过的FE,可以阻止建立真实的相图。我们通过开发一种新的退火方法来克服上述重大问题,称为“解放”,其中单晶在Te蒸气下被退火。具体来说,我们对TE灭绝的超导fe $ _ {1+y} $ te $ _ {1-x} $ se $ _ {x} $进行了各种磁转运测量。我们观察到,从不连贯的到相干电子状态和伪造的开放发生在高温下($ \ $ \ $ \ $ \ $ x $ = 0.2)。在较低温度下具有多带性质的阶段的出现($ \ $ \ $ 50 k,对于$ x $ = 0.2 $ = 0.2)。

Among the Fe-based superconductors, Fe$_{1+y}$Te$_{1-x}$Se$_{x}$ is unique in that its crystal structure is the simplest and the electron correlation level is the strongest, and thus it is important to investigate the doping($x$)-temperature ($T$) phase diagram of this system. However, inevitably incorporated excess Fe currently prevents the establishment of the true phase diagram. We overcome the aforementioned significant problem via developing a new annealing method termed as "Te-annealing" wherein single crystals are annealed under Te vapor. Specifically, we conducted various magnetotransport measurements on Te-annealed superconducting Fe$_{1+y}$Te$_{1-x}$Se$_{x}$. We observed that crossover from the incoherent to the coherent electronic state and opening of the pseudogap occurs at high temperatures ($\approx$ 150 K for $x$ = 0.2). This is accompanied by a more substantial pseudogap and the emergence of a phase with a multi-band nature at lower temperatures (below $\approx$ 50 K for $x$ = 0.2) before superconductivity sets in. Based on the results, the third type electronic phase diagram in Fe-based high-$T_c$ superconductors is revealed.

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