论文标题
染色金属/绝缘子/金属纳米腔的角度和极化选择性自发发射
Angle and Polarization Selective Spontaneous Emission in Dye-doped Metal/Insulator/Metal Nanocavities
论文作者
论文摘要
在基于新兴的纳米发射极技术的新型光子源的角度来看,指导和两极分化荧光团的发射至关重要。这两个任务通常是通过浸入发射极的光学环境的复杂且苛刻的结构来完成的,或者是通过其几何形状和/或带状结构的非平凡的化学工程来完成的。在本文中,证明了在金属/绝缘子/金属(D-MIM)纳米腔中的染料中的波长和极化选择性自发发射。带有大型stokes移位的推扣发色团嵌入在MIM腔中,其共振与发色团的光谱发射带一起调节。角度和极化分辨的光谱实验表明,辐射场根据纳米腔的角度分散重塑,并且其光谱表现出两个带有不同极化对应于该腔的P和S-偏振的谐振的频段。 D-MIM腔是一种高度通用的系统,用于纳米级的极化和波长多路复用应用,以及近场的发射和纳米镜。
Directing and polarizing the emission of a fluorophore is of fundamental importance in the perspective of novel photonic sources based on emerging nano-emitter technologies. These two tasks are usually accomplished by a sophisticated and demanding structuring of the optical environment in which the emitter is immersed, or by non-trivial chemical engineering of its geometry and/or band structure. In this paper, the wavelength and polarization selective spontaneous emission from a dye-embedded in a Metal/Insulator/Metal (d-MIM) nanocavity is demonstrated. A push-pull chromophore with large Stokes shift is embedded in a MIM cavity whose resonances are tuned with the spectral emission band of the chromophore. Angular and polarization resolved spectroscopy experiments reveal that the radiated field is reshaped according to the angular dispersion of the nanocavity, and that its spectrum manifests two bands with different polarization corresponding to the p- and s-polarized resonances of the cavity. The d-MIM cavities are a highly versatile system for polarization and wavelength division multiplexing applications at the nanoscale, as well as for near-field focused emission and nanolenses.