论文标题

镍纳米管的等离子增强原子层沉积,其电阻率低,相干磁化动力学用于3D旋转

Plasma-enhanced atomic layer deposition of nickel nanotubes with low resistivity and coherent magnetization dynamics for 3D spintronics

论文作者

Giordano, M. C., Baumgaertl, K., Steinvall, S. R. Escobar, Gay, J., Vuichard, M., Morral, A. Fontcuberta i, Grundler, D.

论文摘要

我们报告了血浆增强原子层沉积(ALD),以通过使用镍作为前体,水作为氧化剂和周期内等离子体增强氢的氢,以制备共形镍薄膜和纳米管。优化的ALD脉冲序列与后处理后的退火处理相结合,使我们能够在室温下在平面底物和纳米板上准备30 nm厚的金属Ni层,电阻率在室温下为8 $μΩ$ cm。因此,我们制造了几微米长的镍纳米管,直径范围为120至330 nm。我们报告了以磁通量和旋转波模式限制为特征的单个Ni纳米管的ALD生长与功能特性之间的相关性。这些发现为基于3D设备架构的GHz频率制度运行的基于NI的Spintronics和Magnonic设备提供了新的观点。

We report plasma-enhanced atomic layer deposition (ALD) to prepare conformal nickel thin films and nanotubes by using nickelocene as a precursor, water as the oxidant agent and an in-cycle plasma enhanced reduction step with hydrogen. The optimized ALD pulse sequence, combined with a post-processing annealing treatment, allowed us to prepare 30 nm thick metallic Ni layers with a resistivity of 8 $μΩ$cm at room temperature and good conformality both on the planar substrates and nanotemplates. Thereby we fabricated several micrometer-long nickel nanotubes with diameters ranging from 120 to 330 nm. We report on the correlation between ALD growth and functional properties of individual Ni nanotubes characterized in terms of magneto-transport and the confinement of spin wave modes. The findings offer novel perspectives for Ni-based spintronics and magnonic devices operated in the GHz frequency regime with a 3D device architecture.

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