论文标题

通过直接激光写作确定性和可控的光子散射介质

Deterministic and controllable photonic scattering media via direct laser writing

论文作者

Marakis, E., Uppu, R., Meretska, M. L., Gorter, K. J., Vos, W. L., Pinkse, P. W. H.

论文摘要

光子散射材料(例如生物组织和白皮书)是由随机定位的纳米级不均匀性制成的,在折射率中导致光的多重散射。通常,这些材料(无论是天然造成的还是人造的)是通过散射不均匀性的自组装而形成的,这在调整疾病并因此是光学特性时构成了挑战。在这里,我们使用带有确定性设计的直接激光写作报告光子散射介质的纳米化。这些确定性散射介质由亚微米厚聚合物纳米棒组成,这些聚合物纳米棒在立方体积内随机定向。我们使用辐射转移理论研究了光的总传输与杆数密度和样品厚度的函数,以提取散射和传输平均自由路径。具有确定性和可控性能的光子散射介质是基本光散射的模型系统,尤其是具有强各向异性的模型系统,并在固态照明和光伏技术中提供了新的应用。

Photonic scattering materials, such as biological tissue and white paper, are made of randomly positioned nanoscale inhomogeneities in refractive index that lead to multiple scattering of light. Typically these materials, both naturally-occurring or man-made, are formed through self assembly of the scattering inhomogeneities, which imposes challenges in tailoring the disorder and hence the optical properties. Here, We report on the nanofabrication of photonic scattering media using direct laser writing with deterministic design. These deterministic scattering media consist of submicron thick polymer nanorods that are randomly oriented within a cubic volume. We study the total transmission of light as a function of the number density of rods and of the sample thickness to extract the scattering and transport mean free paths using radiative transfer theory. Such photonic scattering media with deterministic and controllable properties are model systems for fundamental light scattering in particular with strong anisotropy and offer new applications in solid-state lighting and photovoltaics.

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